Unveiling PM<sub>2.5</sub> Transport Pathways: A Trajectory-Channel Model Framework for Spatiotemporally Quantitative Source Apportionment

In this study, we introduced a novel Trajectory-Channel Transport Model (TCTM) to unravel spatiotemporal dynamics of PM<sub>2.5</sub> pollution. By integrating high-resolution simulations from the Weather Research and Forecasting (WRF) model with the Nested Air-Quality Prediction Modelin...

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Bibliographic Details
Main Authors: Yong Pan, Jie Zheng, Fangxin Fang, Fanghui Liang, Mengrong Yang, Lei Tong, Hang Xiao
Format: Article
Language:English
Published: MDPI AG 2025-07-01
Series:Atmosphere
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Online Access:https://www.mdpi.com/2073-4433/16/7/883
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Summary:In this study, we introduced a novel Trajectory-Channel Transport Model (TCTM) to unravel spatiotemporal dynamics of PM<sub>2.5</sub> pollution. By integrating high-resolution simulations from the Weather Research and Forecasting (WRF) model with the Nested Air-Quality Prediction Modeling System (WRF-NAQPMS) and 72 h backward-trajectory analysis, TCTM enables the precise identification of source regions, the delineation of key transport corridors, and a quantitative assessment of regional contributions to receptor sites. Focusing on four Yangtze River Delta cities (Hangzhou, Shanghai, Nanjing, Hefei) during a January 2020 pollution event, the results demonstrate that TCTM’s Weighted Concentration Source (WCS) and Source Pollution Characteristic Index (SPCI) outperform traditional PSCF and CWT methods in source-attribution accuracy and resolution. Unlike receptor-based statistical approaches, TCTM reconstructs pollutant transport processes, quantifies spatial decay, and assigns contributions via physically interpretable metrics. This innovative framework offers actionable insights for targeted air-quality management strategies, highlighting its potential as a robust tool for pollution mitigation planning.
ISSN:2073-4433