Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]

Topological insulators (TIs) have unique topologically protected conducting surface and insulating bulk states, which provide a novel platform for plasmonic excitation and related nanoscale functional devices. Exploring plasmon‐enhanced interactions between light and atomic‐layered semiconductors in...

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Main Authors: Yiqiao Zhang, Hua Lu, Zengji Yue, Mingwen Zhang, Xuetao Gan, Jianlin Zhao
Format: Article
Language:English
Published: Wiley-VCH 2025-08-01
Series:Advanced Photonics Research
Subjects:
Online Access:https://doi.org/10.1002/adpr.202400232
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author Yiqiao Zhang
Hua Lu
Zengji Yue
Mingwen Zhang
Xuetao Gan
Jianlin Zhao
author_facet Yiqiao Zhang
Hua Lu
Zengji Yue
Mingwen Zhang
Xuetao Gan
Jianlin Zhao
author_sort Yiqiao Zhang
collection DOAJ
description Topological insulators (TIs) have unique topologically protected conducting surface and insulating bulk states, which provide a novel platform for plasmonic excitation and related nanoscale functional devices. Exploring plasmon‐enhanced interactions between light and atomic‐layered semiconductors in TI nanostructures is particularly significant for optoelectronic applications of TIs. Herein, the Sb2Te3 TI nanotips are fabricated by using focused ion beam lithography technique and the plasmonic hot spot behaviors are investigated on the TI nanotips. The numerical simulation shows that there exists a distinct reinforcement of light field on the Sb2Te3 TI nanotips, which stems from the TI‐based plasmonic hot spot effect. Moreover, the obvious enhancement of photoluminescence (PL) emission from a molybdenum disulfide (MoS2) monolayer integrated onto the Sb2Te3 TI nanotips is experimentally observed. The PL intensity of MoS2 layer on the Sb2Te3 nanotips can be effectively improved by about five‐fold due to the plasmonic hot spot‐induced field reinforcement when compared with that of MoS2 without the Sb2Te3 nanotips. These results will open a new avenue for optoelectronic applications of TIs, especially in nanoscale enhanced PL emission.
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institution Matheson Library
issn 2699-9293
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series Advanced Photonics Research
spelling doaj-art-94a19d7400df40e28a3698d11a9909142025-08-04T08:22:02ZengWiley-VCHAdvanced Photonics Research2699-92932025-08-0168n/an/a10.1002/adpr.202400232Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]Yiqiao Zhang0Hua Lu1Zengji Yue2Mingwen Zhang3Xuetao Gan4Jianlin Zhao5MOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions, and Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Xi'an 710129 ChinaMOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions, and Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Xi'an 710129 ChinaSchool of Artificial Intelligence Science and Technology University of Shanghai for Science and Technology Shanghai 200093 ChinaMOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions, and Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Xi'an 710129 ChinaMOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions, and Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Xi'an 710129 ChinaMOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions, and Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Xi'an 710129 ChinaTopological insulators (TIs) have unique topologically protected conducting surface and insulating bulk states, which provide a novel platform for plasmonic excitation and related nanoscale functional devices. Exploring plasmon‐enhanced interactions between light and atomic‐layered semiconductors in TI nanostructures is particularly significant for optoelectronic applications of TIs. Herein, the Sb2Te3 TI nanotips are fabricated by using focused ion beam lithography technique and the plasmonic hot spot behaviors are investigated on the TI nanotips. The numerical simulation shows that there exists a distinct reinforcement of light field on the Sb2Te3 TI nanotips, which stems from the TI‐based plasmonic hot spot effect. Moreover, the obvious enhancement of photoluminescence (PL) emission from a molybdenum disulfide (MoS2) monolayer integrated onto the Sb2Te3 TI nanotips is experimentally observed. The PL intensity of MoS2 layer on the Sb2Te3 nanotips can be effectively improved by about five‐fold due to the plasmonic hot spot‐induced field reinforcement when compared with that of MoS2 without the Sb2Te3 nanotips. These results will open a new avenue for optoelectronic applications of TIs, especially in nanoscale enhanced PL emission.https://doi.org/10.1002/adpr.202400232molybdenum disulfidephotoluminescencesurface plasmonstopological insulators
spellingShingle Yiqiao Zhang
Hua Lu
Zengji Yue
Mingwen Zhang
Xuetao Gan
Jianlin Zhao
Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
Advanced Photonics Research
molybdenum disulfide
photoluminescence
surface plasmons
topological insulators
title Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
title_full Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
title_fullStr Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
title_full_unstemmed Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
title_short Plasmonic Hot Spots on Topological Insulator Nanotips for Enhancing Light Interaction with MoS2 Atomic Monolayer [invited]
title_sort plasmonic hot spots on topological insulator nanotips for enhancing light interaction with mos2 atomic monolayer invited
topic molybdenum disulfide
photoluminescence
surface plasmons
topological insulators
url https://doi.org/10.1002/adpr.202400232
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AT jianlinzhao plasmonichotspotsontopologicalinsulatornanotipsforenhancinglightinteractionwithmos2atomicmonolayerinvited